This unique framework allows study of energy transport in a synthetic photosynthesis process using a self-assembling peptide-amphiphile (PA) molecule as a scaffold for Zn-porphyrin (ZnP) chromophores.
Significance and impact
Low ratios of ZnP:PA increase spacing in the molecule and improve exciton diffusion, thus linking a controllable parameter to improved light-harvesting capabilities.
- We created samples at the Center for Nanoscale Material (CNM) with varying ratios of ZnP to PA, analyzed all samples with multiple spectroscopy techniques, and studied the exciton diffusion process.
- This study used CNM capabilities: UV/vis, circular dichroism, and electron microscopy as well as time-resolved photoluminescence and transient absorption spectroscopy.
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