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John T. Vaughey

Theme Lead, Senior Chemist

Design, Synthesis, and Characterization of Materials for Energy Storage

Biography

John (Jack) Vaughey is a recognized expert in the design, synthesis, and characterization of next generation materials with applications in energy storage. His current work includes cathode design using oxide, fluoride, and oxyhalide-based materials, battery recycling and upcycling, understanding applications of supply chain to batteries, and silicon (Zintl)-based anode materials. He has over 30 patents covering intermetallic anodes, medical batteries, Mg(Ca)-based energy storage systems, and the Non-Aqueous Organic Redox Flow Batteries for grid storage applications (w A. Jansen, F. Brushett).

Education

  • Northwestern University, Evanston, IL.  Ph.D. Inorganic Materials Chemistry.
  • Worcester Polytechnic Institute, Worcester, MA.  B.Sc. in Chemistry

Awards & Honors

  • Pacesetter Award (ANL) for the Development of the Intermetallic Anode (2000)
  • Outstanding Mentor Award from US Department of Energy, Office of Science (2008)
  • Strategic Laboratory Leadership Program, University of Chicago Booth School of Business (2017-18)
  • Fellow, American Association for the Advancement of Science (2018)

Research & Program Creation 

  • ReCell Battery Recycling
    • ReCell - Co-author/Direct Recycling & Cathode Upcycling Lead Lithium-ion cathodes (2018-pres).
  • High Capacity Anodes
    • Silicon Consortium Program (SCP; TTO) co-PI (2020-pres)
    • Silicon Deep Dive (VTO);  2015-20; PI (2017-20)
    • SEISTA - Solid Electrolyte Interphase Studies on Silicon (VTO) ANL-Lead (2015-2020)
    • BATT (VTO); (1997-2013)
      • Porous All-Inorganic Silicon Electrodes based on metallic copper binders and a CuxSi interfacial compounds
      • Porous Electrode Design for Sb- or Sn-based Intermetallics (including Cu2Sb, Cu6Sn5, InSb)
      • Porous Electrode Design based on nanostructured Li4Ti5O12 anodes
  • JCESR Office of Science Innovation Hub Science;
    • Creator/Author JCESR Beyond Lithium-Ion Program, Multivalent Chemistry (2011-2013, 2018)
    • Creator/Co-author JCESR Grid Storage Program, Non-Aqueous Organic Flow Batteries (2011-13)
    • Co-author/Contributor JCESR Beyond Lithium-Ion Program, Materials Complexity (2018-23)
    • Non-Aqueous Organic Flow Battery: Grid Storage (2005-2012)
      • Demonstrated reversible organic redox flow battery anode materials
      • Several US Patents on the Non-Aqueous Organic Redox Flow Battery (w Andrew Jansen & Fikile Brushett)
  • Integrated Lab Industry Research Program
    • Solid State Batteries & Electrolytes
      • Created multi-lab Solid State Electrolyte-based Battery Program (w John Newman (Berkeley)) with support of EERE/VTO (2009-14)
      • Demonstrated crystal structure control via cation substitutions and processing parameters, pathways of air instability, and identified methods to produce thin LLZO films
      • Determined the Al(III) diffusion pathways (using MAS-NMR, high resolution XRD) that control the phase transitions in Li7La3Zr2O12 garnet solid state electrolytes. 

Professional Service (selected)

  • Associate Editor, Materials Research Bulletin, 2011-present
  • Editorial Board, Chemistry of Materials, 2011-present
  • Electrochemical Society Toyota Young Investigator Award Committee (2017-pres)
  • Electrochemical Society Battery Division Technology Award, Committee (2017-18)
  • The Electrochemical Society, Battery Division, Member-at-Large (2018-22)
  • The Electrochemical Society, Interdisciplinary Science and Technology Subcommitee, (2019-22)
  • Technical Advisory Board, Advanced Materials Research Institute (AMRI), University of New Orleans, New Orleans, LA (2007-2016)
  • AAAS Fellowship Committee (Section C - Chemistry)
  • Symposium Lead Organizer, Beyond Li-Ion Batteries, 232nd Meeting of the Electrochemical Society, National Harbor, MD (2017)
  • Symposium Lead Organizer, Lithium-Ion Batteries and Beyond, 233rd Meeting of the Electrochemical Society, Seattle, WA (2018)
  • Symposium Lead Organizer, Next Generation Battery Materials, 238th Meeting of the Electrochemical Society, Honolulu, HI, (2020).
  • Symposium Lead Organizer, Next Generation Battery Materials, 239th Meeting of the Electrochemical Society, Chicago, IL, (2021)
  • Symposium Lead Organizer, Lithium-Ion Battery Recycling and Safety, 241th Meeting of the Electrochemical Society, Vancouver, BC, (2022).
  • Argonne National Laboratory Directed Research and Development (LDRD) Committee, Chemical Engineering Division, 2005-2008.
  • Argonne Maria Goeppert Meyer Named Fellowship Advisory Committee, co-chair, 2018-2024
  • Argonne Walter Massey Named Fellowship Advisory Committee, co-chair, 2021-2023

Publications and Patents

  • ~200 Publications covering cathodes (lithium-ion, lithium-rich lithium ion, Mg-ion, medical), anodes (lithium metal, intermetallics, silicon), electrolytes (NASICONs, garnets, Mg salts),  and organic flow batteries (materials design)
  • ~30 US Patents on battery, fuel cells, high Tc materials.